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Synthesis and mechanism of a dual-responsive <t>SMP</t> <t>based</t> on PEG. A) Photographs and schematics of shape memory behavior in the PTHF-PEG network, showing two-step programming and recovery due to the crystalline segments of PTHF and PEG (scale bar: 1 cm). Reproduced with permission . Copyright 2021, American Chemical Society. B) Synthetic route of PEG-PLA multiblock copolymer through ring-opening polymerization in the presence of Sn(Oct) 2 as the catalyst. Reproduced with permission . Copyright 2024, Elsevier. C) Schematic illustration of the underlying mechanism of a PLA-PEG copolymer, illustrating the presence of PLA crystalline domains as well as shape recovery due to the temperature- and water-responsiveness of PEG upon exposure to these stimuli. Reproduced with permission . Copyright 2024, Elsevier.
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Synthesis and mechanism of a dual-responsive <t>SMP</t> <t>based</t> on PEG. A) Photographs and schematics of shape memory behavior in the PTHF-PEG network, showing two-step programming and recovery due to the crystalline segments of PTHF and PEG (scale bar: 1 cm). Reproduced with permission . Copyright 2021, American Chemical Society. B) Synthetic route of PEG-PLA multiblock copolymer through ring-opening polymerization in the presence of Sn(Oct) 2 as the catalyst. Reproduced with permission . Copyright 2024, Elsevier. C) Schematic illustration of the underlying mechanism of a PLA-PEG copolymer, illustrating the presence of PLA crystalline domains as well as shape recovery due to the temperature- and water-responsiveness of PEG upon exposure to these stimuli. Reproduced with permission . Copyright 2024, Elsevier.
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Synthesis and mechanism of a dual-responsive SMP based on PEG. A) Photographs and schematics of shape memory behavior in the PTHF-PEG network, showing two-step programming and recovery due to the crystalline segments of PTHF and PEG (scale bar: 1 cm). Reproduced with permission . Copyright 2021, American Chemical Society. B) Synthetic route of PEG-PLA multiblock copolymer through ring-opening polymerization in the presence of Sn(Oct) 2 as the catalyst. Reproduced with permission . Copyright 2024, Elsevier. C) Schematic illustration of the underlying mechanism of a PLA-PEG copolymer, illustrating the presence of PLA crystalline domains as well as shape recovery due to the temperature- and water-responsiveness of PEG upon exposure to these stimuli. Reproduced with permission . Copyright 2024, Elsevier.

Journal: Bioactive Materials

Article Title: Body-responsive shape-memory polymers for biomedical applications

doi: 10.1016/j.bioactmat.2025.12.054

Figure Lengend Snippet: Synthesis and mechanism of a dual-responsive SMP based on PEG. A) Photographs and schematics of shape memory behavior in the PTHF-PEG network, showing two-step programming and recovery due to the crystalline segments of PTHF and PEG (scale bar: 1 cm). Reproduced with permission . Copyright 2021, American Chemical Society. B) Synthetic route of PEG-PLA multiblock copolymer through ring-opening polymerization in the presence of Sn(Oct) 2 as the catalyst. Reproduced with permission . Copyright 2024, Elsevier. C) Schematic illustration of the underlying mechanism of a PLA-PEG copolymer, illustrating the presence of PLA crystalline domains as well as shape recovery due to the temperature- and water-responsiveness of PEG upon exposure to these stimuli. Reproduced with permission . Copyright 2024, Elsevier.

Article Snippet: As noted before, the first successful commercialization of an SMP-based device was Morphix®, which is FDA-cleared as a permanent implant [ , ].

Techniques: